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A favourite of mine is Pulp Fiction. Infact Tarrintino is great with his soundtracks.
Tarantino has a music room that's supposedly the size of a record store, and he has all these rare gems he's collected from around the world which he draws on for inspiration. I think that's why his soundtracks are usually pretty boss - diverse taste in music coupled with a knack for building cool scenes around songs.
Also, maybe I'm being anal-retentive, but are we talking soundtracks and original scores, or just soundtracks, or what? In some cases the two can be completely different animals in the same film.
Big ups to Donnie Darko, soundtrack and score. Some truly wonderful scenes defined by musical choices.
The Edward Scissorhands score music is some of Elfman's greatest work, imo.
I have to say, whether or not Daddy approves, the Velvet Goldmine soundtrack was pretty on point.
Cry-Baby - Bull Moose Jackson? Say no more. Badass original songs, too.
I might catch some flack for this one, but the Clueless soundtrack is a really very nice slice of 90's life.
Eternal Sunshine of the Spotless Mind, mostly score, but that Korgis/Beck scene is kind of gutting.
And, I know it's a TV series, but True Blood has a pretty decent music coordinator.
you're so natural